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A task‐specific mesoporous organic polymer (TSPOP) with unique features like good porosity and rich aromatic phenyl groups was facilely made and utilized as a promising adsorptive desulfurization absorbent for the first time. The material exhibits an efficient saturated adsorption of dibenzothiophene (DBT), as high as 111.1 mg g−1. In addition, the intrinsic mesoporous skeleton of TSPOP gave rise...